Clóves G. Rodrigues, Áurea R. Vasconcellos, José Galvão Ramos, Roberto Luzzi
A Response Function Theory and Scattering Theory applicable to the study of physical properties of systems driven arbitrarily away from equilibrium, specialized for dealing with ultrafast processes and in conditions of space resolution (including nanometric scale), are presented. The derivation is done in the framework of a Gibbs-style Nonequilibrium Statistical Ensemble Formalism. It is shown the connection of the observable properties with time and space-dependent correlation functions out of equilibrium. A generalized fluctuation-dissipation theorem, which relates these correlation functions with generalized susceptibilities is derived. It is also presented the method, useful for calculations, of nonequilibrium-thermodynamic Green functions. A couple of illustration with application of the formalism, consisting of the study of optical responses in ultrafast laser spectroscopy and Raman Scattering of electrons in III-N semiconductors (of "blue diodes") driven away from equilibrium by action of electric fields of moderate to high intensities, are described.
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http://arxiv.org/abs/1210.8108
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